An Investigation of the Chemical Nature of Two Typical by Sherman H. C.

By Sherman H. C.

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Yanisch-Perron C, Viere J, Messing J (1985) Gene, 33: 103 90. Milligan JF, Groebe DR, Witherell GW, Uhlenbeck OC (1987) Nucleic Acids Res, 15: 8783 91. Sampson JR, Uhlenbeck OC (1988) Proc Natl Acad Sci USA, 85: 1033 92. Zuckermann RN, Corey DR, Schultz PG (1988) J Am Chern Soc, 110: 1614 93. James BD, Olsen GJ, Lieu J, Pace NR (1988) Cell, 52: 19 94. Stern S, Weiser B, Noller HE (1988) J Mol Bioi, 204: 447 95. Blackburn P, Moore S (1982) The Enzymes, 3rd edition, 15: 317 96. Erman JE, Hammes GGJ (1966) Am Chern Soc, 88: 5614 97.

3 Structure of Molecular Tweezers. . . . . . . . . . . . . 4 Complexation by Molecular Tweezers. . . . . . . . . . . 45 45 46 47 50 5 Complexation of Nucleotide Bases Using Hydrogen Bonding and n-Stacking. . . . . . . . . . . . . . . . . . .. 1 Introduction...... . . . . . . . . . . . . . . . . . .. 2 Receptors That Use Only Hydrogen Bonding Forces. . . . . 3 Receptors That Use Hydrogen Bonding Forces and a Single n-Stacking Interaction .

60 60 62 66 6 Summary and Future Directions. . . . . . . . . . . . . . . 69 7 Acknowledgements . . . . . . . . . . . . . . . . . . . . 70 8 References. . . . . . . . . . . . . . . . . . . . . . . .. 70 Synthetic Receptors for n-Sandwich Complexation of Aromatic Substrates 35 1 Introduction The proper functioning of any organism depends upon an extraordinary organization of biochemical systems. On a molecular level, this organization is seen in the well defined three dimensional structure which most biopolymers adopt, and in the high affinity, and often exquisite selectivity, with which macromolecules interact with other molecules, both large and small.

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